Repositorio Institucional del CAB-IB

Coltrims - espectroscopía de iones en retroceso aplicada al estudio de captura selectiva en colisiones 3"He"2+ + He y He"+ + H_2 a energías intermedias de colisión. / Coltrims - a state selective electron capture study por 3"He"2+ + He and He"+ + H_2 collisions at intermediate collision energies using the recoil ion momentum spectroscopy technique.

Alessi, Mariana (2012) Coltrims - espectroscopía de iones en retroceso aplicada al estudio de captura selectiva en colisiones 3"He"2+ + He y He"+ + H_2 a energías intermedias de colisión. / Coltrims - a state selective electron capture study por 3"He"2+ + He and He"+ + H_2 collisions at intermediate collision energies using the recoil ion momentum spectroscopy technique. Tesis Doctoral en Física, Universidad Nacional de Cuyo, Instituto Balseiro.

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Resumen en español

En este trabajo se realizó el montaje, puesta en funcionamiento y caracterización del nuevo sistema COLTRIMS (Cold Target Recoil-Ion Momentum Spectroscopy), en la División Colisiones Atómicas en el Centro Atómico Bariloche. Se desarrolló el método y programa de procesamiento de datos y ampliación del programa de adquisición, de dicho equipamiento. Y finalmente se realizó un estudio experimental, con acompañamiento teórico, de procesos de colisiones en sistemas ion-átomo e ion-molécula. En particular, el estudio se enfocó en estados selectivos de captura simple, en los sistemas 3"He"2+ + He y He"+ + H_2, respectivamente, en un rango de energías intermedias de colisión, comprendido entre 13.3 - 100 keV/amu, para el primer sistema y 6.25 - 50 keV/amu para el segundo. Los resultados obtenidos en 3"He"2+ + He, abordan un rango de energías no estudiado por otros laboratorios. Asimismo, para el sistema He"+ + H_2, se consideró un proyectil parcialmente ionizado, prácticamente inexplorado teórica y experimentalmente. En ambos casos, se midieron las distribuciones de captura a diferentes estados del blanco y del proyectil. Dicho estudio, se obtiene a partir de las mediciones de las distribuciones de momentos longitudinales con valores inferiores a 1 a.u., de los iones resultantes de la colisión. Se determinó el momento transversal total de los iones, implementando un procedimiento que basado en argumentos de simetría, permite obtener dicha distribución a partir de la componente transversal del momento medida en una dirección. Para ambos sistemas, los resultados experimentales fueron normalizados y contrastados con resultados teóricos obtenidos por modelos clásicos de Monte Carlo, de cuatro cuerpos con inclusión de apantallamiento dinámico de los electrones (dCTMC), para el caso ion-átomo y de cinco cuerpos CTMC, para el sistema ion-molécula. Completando el estudio de la cinemática, a partir de los momentos transversales de los iones en retroceso, se obtuvo el ángulo de scattering del proyectil para ángulos menores a 1 mrad, prácticamente inaccesibles para otro tipo de espectroscopía.

Resumen en inglés

In this work we performed the installation, the set-up and characterization of the new COLTRIMS device (Cold Target Recoil-Ion Momentum Spectroscopy), at the Atomic Collisions Division of the Centro Atómico Bariloche. We developed the method, the data processing program and the expansion of the acquisition program, for this equipment. And finally, we performed an experimental study, with theoretical discussions, of collision processes in ion-atom and ion-molecule systems. In particular, the study was focused on state selective electron capture, for the 3"He"2+ + He and He+ + H_2 collisions systems, at intermediate energy ranges of 13.3 - 100 keV/amu and 6.25 - 50 keV/amu, respectively. The obtained results for the 3He2+ + He system, consider an energy range that has not been studied by other laboratories before. Besides, for the He"+ + H_2 system, a dressed projectile was considered, a case practically unexplored in former theoretical and experimental studies. In both cases, the capture distributions for different states of the target and the projectile were measured. This study was obtained from measurements of the longitudinal momentum distributions of the resulting ions from the collisions with values less than 1 a.u.. We also determined the total transversal momentum of the recoiling ions, implementing a procedure based on symmetry arguments, that allows to obtain such distribution from the transversal momentum component measured in one direction. For both systems, the experimental results were normalized and compared to theoretical results obtained by classical Monte Carlo models, of four bodies including dynamic screening of the electrons (dCTMC), in the case of ion-atom and five bodies CTMC, for ion-molecule system. Completing the kinematics study, we obtained the scattering angle of the projectile for angles less than 1 mrad, from the transversal momentum of the recoil ions, practically inaccessible to other types of spectroscopy.

Tipo de objeto:	Tesis (Tesis Doctoral en Física)
Palabras Clave:	Electron capture; Captura electrónica; Position sensitive detectors; Detectores de localización; Helium; Helio; Coltrims; Cold target recoil-ion momentum spectroscopy; Selective capture; Captura selectiva; Molecular hydrogen; Hidrógeno Molecular
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Materias:	Física
Divisiones:	Investigación y aplicaciones no nucleares > Física > Colisiones atómicas
Código ID:	400
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